The coexistence of phases, characterized by different electronic degrees of freedom, commonly occurs in layered superconductors. Among them, alkaline intercalated chalcogenides are model systems showing the microscale coexistence of paramagnetic (PAR) and antiferromagnetic (AFM) phases, however, the temporal behavior of different phases is still unknown. Here, we report a visualization of the atomic motion in the granular phase of KxFe2-ySe2 using x-ray photon correlation spectroscopy. Unlike the PAR phase, the AFM texture reveals an intermittent dynamics with avalanches as in martensites. When cooled down across the superconducting transition temperature T-c, the AFM phase goes through an anomalous slowing behavior, suggesting a direct relationship between the atomic motions in the AFM phase and the superconductivity. In addition to providing compelling evidence of avalanchelike dynamics in a layered superconductor, the results provide a basis for different theoretical models to describe the quantum states in inhomogeneous solids.

Intermittent dynamics of antiferromagnetic phase in inhomogeneous iron-based chalcogenide superconductor

Campi, G.;Saini, N. L.
2020

Abstract

The coexistence of phases, characterized by different electronic degrees of freedom, commonly occurs in layered superconductors. Among them, alkaline intercalated chalcogenides are model systems showing the microscale coexistence of paramagnetic (PAR) and antiferromagnetic (AFM) phases, however, the temporal behavior of different phases is still unknown. Here, we report a visualization of the atomic motion in the granular phase of KxFe2-ySe2 using x-ray photon correlation spectroscopy. Unlike the PAR phase, the AFM texture reveals an intermittent dynamics with avalanches as in martensites. When cooled down across the superconducting transition temperature T-c, the AFM phase goes through an anomalous slowing behavior, suggesting a direct relationship between the atomic motions in the AFM phase and the superconductivity. In addition to providing compelling evidence of avalanchelike dynamics in a layered superconductor, the results provide a basis for different theoretical models to describe the quantum states in inhomogeneous solids.
2020
Istituto di Cristallografia - IC
Inglese
101
2
5
https://journals.aps.org/prb/abstract/10.1103/PhysRevB.101.020508
Esperti anonimi
Superconductivity
Disordered systems
X ray Photon Correlation Spectroscopy
Internazionale
12
info:eu-repo/semantics/article
262
Ricci, A.; Campi, G.; Joseph, B.; Poccia, N.; Innocenti, D.; Gutt, C.; Tanaka, M.; Takeya, H.; Takano, Y.; Mizokawa, T.; Sprung, M.; Saini, N. L....espandi
01 Contributo su Rivista::01.01 Articolo in rivista
none
File in questo prodotto:
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/380943
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 11
  • ???jsp.display-item.citation.isi??? 10
social impact