We present a novel approximation scheme to describe the influence of a harmonic bath on the dynamics of a two-level particle over almost the whole regime of temperatures and coupling to the environment, for a wide class of bath spectral densities. Starting from the exact path integral solution for the two-level system density matrix, effective intra-blip correlations are fully included, while inter-blip and blip-sojourn interactions are considered up to first order. In the proper regimes, an excellent agreement with conventional perturbative approaches and ab initio path-integral results is found. Copyright (c) EPLA, 2007.

Spin-boson dynamics: A unified approach from weak to strong coupling

Paladino E;
2007

Abstract

We present a novel approximation scheme to describe the influence of a harmonic bath on the dynamics of a two-level particle over almost the whole regime of temperatures and coupling to the environment, for a wide class of bath spectral densities. Starting from the exact path integral solution for the two-level system density matrix, effective intra-blip correlations are fully included, while inter-blip and blip-sojourn interactions are considered up to first order. In the proper regimes, an excellent agreement with conventional perturbative approaches and ab initio path-integral results is found. Copyright (c) EPLA, 2007.
2007
INFM
TUNNELING DYNAMICS
OHMIC DISSIPATION
ELECTRON-TRANSFER
2-LEVEL SYSTEM
QUANTUM-STATE
File in questo prodotto:
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/159324
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus ND
  • ???jsp.display-item.citation.isi??? ND
social impact