The frequency-reduced representation, g(omega)/omega(2). of the vibrational density of states g(a)), known as the Boson peak is frequency used to extract information Oil structural and dynamical properties of glasses and supercooled liquids. The g(omega)/omega(2) representation is preferred over the true excess of the vibrational modes, defined as the difference between the total g(omega) and the Debye contribution, for practical reasons. Analysis of a large body of the available experimental data from inelastic neutron and Raman scattering reveals that reduction procedures distort to a great extent the otherwise symmetric excess density of states. The frequency and the intensity of the Boson peak are very sensitive to minor modifications of the distribution of the excess. The quantitative Use Of the 11(omega)/(omega)(2) function leads to sonic peculiar results that contradict our general perception about glass-forming materials. We stress that the structure and dynamics of. physics of the low-energy excitations are hidden in the excess density of states, Which should attract more attention both from the experimental Lis well Lis the theoretical point of view.
Some remarks on the low-energy excitations in glasses: interpretation of Boson peak data
Ruocco G
2007
Abstract
The frequency-reduced representation, g(omega)/omega(2). of the vibrational density of states g(a)), known as the Boson peak is frequency used to extract information Oil structural and dynamical properties of glasses and supercooled liquids. The g(omega)/omega(2) representation is preferred over the true excess of the vibrational modes, defined as the difference between the total g(omega) and the Debye contribution, for practical reasons. Analysis of a large body of the available experimental data from inelastic neutron and Raman scattering reveals that reduction procedures distort to a great extent the otherwise symmetric excess density of states. The frequency and the intensity of the Boson peak are very sensitive to minor modifications of the distribution of the excess. The quantitative Use Of the 11(omega)/(omega)(2) function leads to sonic peculiar results that contradict our general perception about glass-forming materials. We stress that the structure and dynamics of. physics of the low-energy excitations are hidden in the excess density of states, Which should attract more attention both from the experimental Lis well Lis the theoretical point of view.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.