Resistivity under pressure and magnetization measurements on Ba1-xSrxVS3 single crystals with 0 x 0.18 and no sulphur deficiency show an abrupt onset of ferromagnetic (FM) order at a critical value x=0.07, concomitant to a change of the magnetic properties at the metal-insulator transition (MIT) and to a collapse of the unit cell at ambient temperature. A reduction of the MIT temperature to 50 K upon x that scales as the V-S distance is also observed. This gives evidence of a chemical pressure induced quantum phase transition that stabilizes the incipient FM order of BaVS3. The 0.07 < x results suggest a coexistence of FM and metallic phases at larger x.

Evidence of ferromagnetic quantum phase transition in Ba1-xSrxVS3

F Licci;F Bolzoni;E Gilioli;
2006

Abstract

Resistivity under pressure and magnetization measurements on Ba1-xSrxVS3 single crystals with 0 x 0.18 and no sulphur deficiency show an abrupt onset of ferromagnetic (FM) order at a critical value x=0.07, concomitant to a change of the magnetic properties at the metal-insulator transition (MIT) and to a collapse of the unit cell at ambient temperature. A reduction of the MIT temperature to 50 K upon x that scales as the V-S distance is also observed. This gives evidence of a chemical pressure induced quantum phase transition that stabilizes the incipient FM order of BaVS3. The 0.07 < x results suggest a coexistence of FM and metallic phases at larger x.
2006
Istituto dei Materiali per l'Elettronica ed il Magnetismo - IMEM
71.30.+h
71.27.+a
75.50.-y
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/182361
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