High-time-resolution broadband pump-probe spectroscopy of rhodopsin reveals the loss of reactant and appearance of photoproduct features within approximate to 100fs, which are signatures of a wavepacket moving through a conical intersection. Experiments are supported by molecular dynamics simulations. (C) Optical Society of America
Direct Observation of the Conical Intersection in cis-trans Photoisomerization of Rhodopsin
Manzoni;Cristian;Cerullo;Giulio;
2009
Abstract
High-time-resolution broadband pump-probe spectroscopy of rhodopsin reveals the loss of reactant and appearance of photoproduct features within approximate to 100fs, which are signatures of a wavepacket moving through a conical intersection. Experiments are supported by molecular dynamics simulations. (C) Optical Society of AmericaFile in questo prodotto:
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