A very accurate method is applied, within the theoretical framework of the scattering close-coupling equations, to treat rotational predissociation processes in the He-CO van der Waals molecule. The method was already employed successfully to study vibrational predissociation of the He-I*2 complexes and shows in the present case significant differences with several approximate methods used to estimate resonance positions. The physical implications of such differences are analyzed and discussed.
Rotational predissociation of strongly anisotropic Van der Waals complexes: the He - CO example.
A Palma
1987
Abstract
A very accurate method is applied, within the theoretical framework of the scattering close-coupling equations, to treat rotational predissociation processes in the He-CO van der Waals molecule. The method was already employed successfully to study vibrational predissociation of the He-I*2 complexes and shows in the present case significant differences with several approximate methods used to estimate resonance positions. The physical implications of such differences are analyzed and discussed.File in questo prodotto:
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