We present the main features of CITIUS, a new light source for ultrafast science, generating tunable, intense, femtosecond pulses in the spectral range from IR to XUV. The XUV pulses (about 105-108 photons/pulse in the range 14-80 eV) are produced by laser-induced high-order harmonic generation in gas. This radiation is monochromatized by a time-preserving monochromator, allowing also to work with high-resolution andwidth selection. The tunable IR-UV pulses (1012--1015 photons/pulse in the range 0.4-5.6 eV) are generated by an optical parametric amplifier, which is driven by a fraction of the same laser pulse that enerates high order harmonics. The IR-UV and XUV pulses follow dierent optical paths and are eventually recombined on the ample for pump-probe experiments. The new light source will become the fulcrum of a new center located at the University of Nova Gorica, active in a wide range of scientific fields, including materials science, catalysis, biochemistry and magnetism. We also present the results of two pump-probe experiments: with the first one, we fully characterized the temporal duration of harmonic pulses in the time-preserving configuration; with the second one, we demonstrated the possibility of using CITIUS for selective investigation of the ultra-fast dynamics of dierent elements in a magnetic compound.

CITIUS: An infrared-extreme ultraviolet light source for fundamental and applied ultrafast science

C Grazioli;M Coreno;F Frassetto;A Kivimaki;P Miotti;L Poletto;E Polo;
2014

Abstract

We present the main features of CITIUS, a new light source for ultrafast science, generating tunable, intense, femtosecond pulses in the spectral range from IR to XUV. The XUV pulses (about 105-108 photons/pulse in the range 14-80 eV) are produced by laser-induced high-order harmonic generation in gas. This radiation is monochromatized by a time-preserving monochromator, allowing also to work with high-resolution andwidth selection. The tunable IR-UV pulses (1012--1015 photons/pulse in the range 0.4-5.6 eV) are generated by an optical parametric amplifier, which is driven by a fraction of the same laser pulse that enerates high order harmonics. The IR-UV and XUV pulses follow dierent optical paths and are eventually recombined on the ample for pump-probe experiments. The new light source will become the fulcrum of a new center located at the University of Nova Gorica, active in a wide range of scientific fields, including materials science, catalysis, biochemistry and magnetism. We also present the results of two pump-probe experiments: with the first one, we fully characterized the temporal duration of harmonic pulses in the time-preserving configuration; with the second one, we demonstrated the possibility of using CITIUS for selective investigation of the ultra-fast dynamics of dierent elements in a magnetic compound.
2014
Istituto di fotonica e nanotecnologie - IFN
Istituto per la Sintesi Organica e la Fotoreattivita' - ISOF
Istituto di Struttura della Materia - ISM - Sede Roma Tor Vergata
Istituto Officina dei Materiali - IOM -
infrared
ultraviolet
light source
ultrafast science
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/254022
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