Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system - a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast electronic charge transfer.
Quantum coherence controls the charge separation in a prototypical artificial light harvesting system
Rozzi C A;Spallanzani N;
2013
Abstract
Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system - a supramolecular triad - provide strong evidence that the quantum-correlated wavelike motion of electrons and nuclei on a timescale of few tens of femtoseconds governs the ultrafast electronic charge transfer.File in questo prodotto:
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