The ion dynamics of a saturated lithium ammonia solution was investigated by inelastic neutron scattering with optimized resolution. The experimental dispersion curve and mode damping, here carefully probed in a wave-vector range extending well below and above 1 angstrom(-1), display visible anomalies around 0.8 angstrom(-1). We relate the dispersion relation anomaly to the shape of the electron gas dielectric function, which screens the ion-ion potential in a way peculiar of the low electron density of the system. The increase of the damping around 0.8 angstrom(-1) also supports the presence of a new decay channel for the collective excitations. An interpretation of these effects, based on the low electron-density properties of the lithium-ammonia solution, is proposed.

Collective modes in a saturated lithium-ammonia solution as a probe of the response of the low-density homogeneous electron gas

Petrillo C;Sacchetti F;
2011

Abstract

The ion dynamics of a saturated lithium ammonia solution was investigated by inelastic neutron scattering with optimized resolution. The experimental dispersion curve and mode damping, here carefully probed in a wave-vector range extending well below and above 1 angstrom(-1), display visible anomalies around 0.8 angstrom(-1). We relate the dispersion relation anomaly to the shape of the electron gas dielectric function, which screens the ion-ion potential in a way peculiar of the low electron density of the system. The increase of the damping around 0.8 angstrom(-1) also supports the presence of a new decay channel for the collective excitations. An interpretation of these effects, based on the low electron-density properties of the lithium-ammonia solution, is proposed.
2011
Istituto Officina dei Materiali - IOM -
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/322452
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