The collective dynamics of liquid rubidium was measured by inelastic neutron scattering from melting up to 1673 K and 6.4 MPa to explore an electron gas instability, forecasted by theory at sufficient expansion. Pronounced variations are observed when the predicted conditions are approached. They comply with a scenario for the density-driven metal-to-non-metal transition suggested for fluid mercury where the liquid metal decomposes into a nanoemulsion of metallic and non-metallic domains and the metallic domains constantly disappear with ongoing expansion. Collective modes appear as an unambiguous signature of the metallic phase allowing to directly observe this process. © CopyrightEPLA, 2018.

New perspectives onto the metal-to-non-metal transition in expanded liquid metals

Orecchini A;Laloni A;De Francesco A
2018

Abstract

The collective dynamics of liquid rubidium was measured by inelastic neutron scattering from melting up to 1673 K and 6.4 MPa to explore an electron gas instability, forecasted by theory at sufficient expansion. Pronounced variations are observed when the predicted conditions are approached. They comply with a scenario for the density-driven metal-to-non-metal transition suggested for fluid mercury where the liquid metal decomposes into a nanoemulsion of metallic and non-metallic domains and the metallic domains constantly disappear with ongoing expansion. Collective modes appear as an unambiguous signature of the metallic phase allowing to directly observe this process. © CopyrightEPLA, 2018.
2018
Istituto Officina dei Materiali - IOM -
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/354440
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