The air-exposed hydrogenated diamond surface has been studied by carrier transport measurements and density functional theory. Our results have allowed us to understand the close relationship between the physisorbed water molecules and the electrical resistance. We have therefore been able to show that the evolution of the resistance over time and temperature can be related to the extent of the hole accumulation layer originating at the surface of the hydrogenated diamond. The method has allowed us to estimate the desorption energy of a single water molecule by means of resistance measurements alone.

Water desorption effects on the surface electrical resistance of air-exposed hydrogenated diamond

Flammini R;Satta M;Bellucci A;Girolami M;Trucchi DM
2020

Abstract

The air-exposed hydrogenated diamond surface has been studied by carrier transport measurements and density functional theory. Our results have allowed us to understand the close relationship between the physisorbed water molecules and the electrical resistance. We have therefore been able to show that the evolution of the resistance over time and temperature can be related to the extent of the hole accumulation layer originating at the surface of the hydrogenated diamond. The method has allowed us to estimate the desorption energy of a single water molecule by means of resistance measurements alone.
2020
Istituto di Struttura della Materia - ISM - Sede Roma Tor Vergata
Istituto di Struttura della Materia - ISM - Sede Secondaria Montelibretti
Istituto per lo Studio dei Materiali Nanostrutturati - ISMN
diamond
hydrogenated diamond
electrical conductivity
DFT
desorption energy
water molecule
charge transfer
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/363360
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