By means of infrared spectroscopy, we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba1-xKxFe2As2. The Fano parameter 1/q2, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic and structural orderings at low temperatures. Most strikingly, at elevated temperatures in the paramagnetic tetragonal state we observe a linear correlation between 1/q2 and the superconducting critical temperature Tc. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable xy orbital component at the Fermi level is fundamental for the Fano effect and, thus, possibly also for the superconducting pairing.

Scaling of the Fano Effect of the In-Plane Fe-As Phonon and the Superconducting Critical Temperature in Ba1-x KxFe2As2

Cappelluti, E.;Benfatto, L.;
2019

Abstract

By means of infrared spectroscopy, we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba1-xKxFe2As2. The Fano parameter 1/q2, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic and structural orderings at low temperatures. Most strikingly, at elevated temperatures in the paramagnetic tetragonal state we observe a linear correlation between 1/q2 and the superconducting critical temperature Tc. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable xy orbital component at the Fermi level is fundamental for the Fano effect and, thus, possibly also for the superconducting pairing.
2019
Istituto di Struttura della Materia - ISM - Sede Roma Tor Vergata
Istituto dei Sistemi Complessi - ISC
Barium compounds
Infrared spectroscopy
Iron compounds
PhononsTemperature
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/364759
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