The presence of lattice correlated disorder in real materials places further demands on the understanding of structure-function relationship. The study of this disorder is quite challenging since it can be due to various and interconnected reasons. This requires advanced probes able to measure weak structural features. Thanks to synchrotron radiation features is nowadays possible to visualize structural disorder alongside its spatial distribution and time dynamics. In this context we aim to characterize thin film superconducting YBa2Cu3O7-x whose structure is particularly rich. Indeed, here the nano-granularity related to super-lattices, distribution of dopants, strain induced stoichiometry inhomogeneity, are coupled with the intrinsic granularity arising from the material island growth mode, which leads to small grains (~200 nm) and a large network of grain boundaries (GB). X-ray Grazing incidence diffraction has been used to visualize low dimensional lattice disorder in optimally doped YBa2Cu3O7-x with inclusion of BaZrO3 nanodefects grown on SrTiO3 single crystals. The results are expected to shade light on interplay of lattice disorder and the electronic quantum coherence in the superconducting state.
Correlated disorder in YBCO and composite YBCO films revealed by means of synchrotron X-ray diffraction
Luisa Barba;Gianmichele Arrighetti;Gaetano Campi
2018
Abstract
The presence of lattice correlated disorder in real materials places further demands on the understanding of structure-function relationship. The study of this disorder is quite challenging since it can be due to various and interconnected reasons. This requires advanced probes able to measure weak structural features. Thanks to synchrotron radiation features is nowadays possible to visualize structural disorder alongside its spatial distribution and time dynamics. In this context we aim to characterize thin film superconducting YBa2Cu3O7-x whose structure is particularly rich. Indeed, here the nano-granularity related to super-lattices, distribution of dopants, strain induced stoichiometry inhomogeneity, are coupled with the intrinsic granularity arising from the material island growth mode, which leads to small grains (~200 nm) and a large network of grain boundaries (GB). X-ray Grazing incidence diffraction has been used to visualize low dimensional lattice disorder in optimally doped YBa2Cu3O7-x with inclusion of BaZrO3 nanodefects grown on SrTiO3 single crystals. The results are expected to shade light on interplay of lattice disorder and the electronic quantum coherence in the superconducting state.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.