Stabilised dense emulsions display a rich phenomenology connecting microstructure and rheology. In this work, we study how an emulsion with a finite yield stress can be built via large-scale stirring. By gradually increasing the volume fraction of the dispersed minority phase, under the constant action of a stirring force, we are able to achieve a volume fraction close to 80%. Despite the fact that our system is highly concentrated and not yet turbulent we observe a droplet size distribution consistent with the -10/3 scaling, often associated with inertial range droplets breakup. We report that the polydispersity of droplet sizes correlates with the dynamics of the emulsion formation process. Additionally, we quantify the visco-elastic properties of the dense emulsion finally obtained and we demonstrate the presence of a finite yield stress. The approach reported can pave the way to a quantitative understanding of the complex interplay between the dynamics of mesoscale constituents and the large-scale flow properties of yield stress fluids.

Build up of yield stress fluids via chaotic emulsification

Scagliarini;Andrea;Toschi;Federico
2022

Abstract

Stabilised dense emulsions display a rich phenomenology connecting microstructure and rheology. In this work, we study how an emulsion with a finite yield stress can be built via large-scale stirring. By gradually increasing the volume fraction of the dispersed minority phase, under the constant action of a stirring force, we are able to achieve a volume fraction close to 80%. Despite the fact that our system is highly concentrated and not yet turbulent we observe a droplet size distribution consistent with the -10/3 scaling, often associated with inertial range droplets breakup. We report that the polydispersity of droplet sizes correlates with the dynamics of the emulsion formation process. Additionally, we quantify the visco-elastic properties of the dense emulsion finally obtained and we demonstrate the presence of a finite yield stress. The approach reported can pave the way to a quantitative understanding of the complex interplay between the dynamics of mesoscale constituents and the large-scale flow properties of yield stress fluids.
2022
Istituto Applicazioni del Calcolo ''Mauro Picone''
Inglese
23
6
1
11
Sì, ma tipo non specificato
Turbulent emulsions
turbulence
emulsions
2
info:eu-repo/semantics/article
262
Girotto; Ivan;Benzi; Roberto;Di Staso; Gianluca;Scagliarini; Andrea;Schifano; Sebastiano Fabio;Toschi; Federico
01 Contributo su Rivista::01.01 Articolo in rivista
none
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/413696
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