We present a self-mixing intermode-beatnote spectroscopy system, based on a THz quantum cascade laser operating as a frequency comb (FC). The emitted radiation is back-scattered from the tip of a scanning near-field opticalmicroscope (s-SNOM), which allows to exploit the sensitivity of FC phase-coherence to optical feedback to manipulate the frequency, amplitude and linewidth of the intermode FC beatnote. By stabilizing the phase-locked regimes, we demonstrate, for the first time, a FC based hyper-spectral, THz sSNOM nanoscope providing coherent detection of multiple phase-locked modes and mapping of the THz near-field response of materials in the 2.29-3.6 THz range, with noise-equivalentpowers of similar to 400pW/vHz.

Phase-sensitive hyperspectral near-field nanoscope based on self-induced phase locking of terahertz frequency combs

Pistore, Valentino;Pogna, Eva;Viti, Leonardo;Vitiello, Miriam S.
2022

Abstract

We present a self-mixing intermode-beatnote spectroscopy system, based on a THz quantum cascade laser operating as a frequency comb (FC). The emitted radiation is back-scattered from the tip of a scanning near-field opticalmicroscope (s-SNOM), which allows to exploit the sensitivity of FC phase-coherence to optical feedback to manipulate the frequency, amplitude and linewidth of the intermode FC beatnote. By stabilizing the phase-locked regimes, we demonstrate, for the first time, a FC based hyper-spectral, THz sSNOM nanoscope providing coherent detection of multiple phase-locked modes and mapping of the THz near-field response of materials in the 2.29-3.6 THz range, with noise-equivalentpowers of similar to 400pW/vHz.
2022
Istituto Nanoscienze - NANO
Photomapping, Quantum cascade lasers, Terahertz spectroscopy, Terahertz waves
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/418744
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