The dipolar approximation model that describes the heat delivered by a nanoparticle under continuous light irradiation provides a relation in which the dissipated power is proportional to the extinction cross-section. This relation works fairly well for small particles in which all the energy is absorbed, but fails for larger structures due to the non-negligible power scattered in the free space that does not contribute to heat generation. Here we show that, if we consider the light-induced dipolar field in the calculation of the dissipated power, we recover the proportionality with the absorption cross-section of the nanoparticle.
Heat Dissipation of Metal Nanoparticles in the Dipole Approximation
Gillibert Raymond;Gucciardi Pietro G
2020
Abstract
The dipolar approximation model that describes the heat delivered by a nanoparticle under continuous light irradiation provides a relation in which the dissipated power is proportional to the extinction cross-section. This relation works fairly well for small particles in which all the energy is absorbed, but fails for larger structures due to the non-negligible power scattered in the free space that does not contribute to heat generation. Here we show that, if we consider the light-induced dipolar field in the calculation of the dissipated power, we recover the proportionality with the absorption cross-section of the nanoparticle.File in questo prodotto:
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