We present a model of the electronic transport in a nanotube quantum dot coupled with local phonon modes and with the leads. The Hamiltonian model is analysed by means of a variational approach that is accurate in the whole regime of the coupling parameters. The method, while reproducing the standard solution for limit values of the coupling parameters (e.g. the adiabatic limit), includes the effects of dynamical distortion and the fluctuations of phonon modes. These effects are important to obtain a more accurate approximation of the system quantum state away from these limits. Unusual electrical features, i.e. negative differential resistance, switching and hysteresis, emerge from the current-voltage characteristic of this model molecular device. However, the quantum corrections modify substantially the transport scenario away from the adiabatic limit. In particular, fluctuations and polaronic distortion contrast the bi-stability of the solution, which is evidenced by the Born-Oppenheimer analysis. As a consequence, our method correctly foresees the anomalous transport features and their dependence on the Hamiltonian parameters and biasing regimes. (C) 2007 Elsevier B.V. All rights reserved.
A polaron model of the electronic transport in a nanotube quantum dot
La Magna A;Deretzis I
2008
Abstract
We present a model of the electronic transport in a nanotube quantum dot coupled with local phonon modes and with the leads. The Hamiltonian model is analysed by means of a variational approach that is accurate in the whole regime of the coupling parameters. The method, while reproducing the standard solution for limit values of the coupling parameters (e.g. the adiabatic limit), includes the effects of dynamical distortion and the fluctuations of phonon modes. These effects are important to obtain a more accurate approximation of the system quantum state away from these limits. Unusual electrical features, i.e. negative differential resistance, switching and hysteresis, emerge from the current-voltage characteristic of this model molecular device. However, the quantum corrections modify substantially the transport scenario away from the adiabatic limit. In particular, fluctuations and polaronic distortion contrast the bi-stability of the solution, which is evidenced by the Born-Oppenheimer analysis. As a consequence, our method correctly foresees the anomalous transport features and their dependence on the Hamiltonian parameters and biasing regimes. (C) 2007 Elsevier B.V. All rights reserved.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.
