The two-dimensional electron system (2DES) located at the surface of strontium titanate (STO) and at several other STO-based interfaces has been an established platform for the study of novel physical phenomena since its discovery. Here we report how the interfacing of STO and tetracyanoquinodimethane (TCNQ) results in a charge transfer that depletes the number of free carriers at the STO surface, with a strong impact on its electronic structure. Our study paves the way for efficient tuning of the electronic properties, which promises novel applications in the framework of oxide/organic-based electronics.
Charge Transfer and Orbital Reconstruction at an Organic-Oxide Interface
Schio L.;Verdini A.;Floreano L.;
2023
Abstract
The two-dimensional electron system (2DES) located at the surface of strontium titanate (STO) and at several other STO-based interfaces has been an established platform for the study of novel physical phenomena since its discovery. Here we report how the interfacing of STO and tetracyanoquinodimethane (TCNQ) results in a charge transfer that depletes the number of free carriers at the STO surface, with a strong impact on its electronic structure. Our study paves the way for efficient tuning of the electronic properties, which promises novel applications in the framework of oxide/organic-based electronics.File in questo prodotto:
| File | Dimensione | Formato | |
|---|---|---|---|
|
caputo-et-al-2023-charge-transfer-and-orbital-reconstruction-at-an-organic-oxide-interface_ok.pdf
Open Access dal 01/12/2024
Descrizione: This document is the Accepted Manuscript version of a Published Work that appeared in final form in Nano Letters, Copyright ©2023 American Chemical Society, after peer review and technical editing by the publisher.
Tipologia:
Documento in Post-print
Licenza:
Altro tipo di licenza
Dimensione
1.19 MB
Formato
Adobe PDF
|
1.19 MB | Adobe PDF | Visualizza/Apri |
I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.
