Two-dimensional electronic spectroscopy (2DES) is a popular technique that can track ultrafast coherent and incoherent processes in real time. Since its development in the late 1990s, 2DES has become a powerful tool for investigating ultrafast dynamics in a range of systems, including nanomaterials and optoelectronic devices. This Primer explains the underlying physical principles of 2DES and how it can be applied to study dynamic photophysical processes. The article discusses how to collect, process and analyse data, with a summary of currently available experimental configurations. Common issues and challenges are considered, focusing on the limitations and reproducibility of the technique, finishing with an exploration of potential future advances and applications.
Two-dimensional electronic spectroscopy
Valduga de Almeida Camargo F.Secondo
Writing – Original Draft Preparation
;Cerullo G.Penultimo
Writing – Original Draft Preparation
;
2023
Abstract
Two-dimensional electronic spectroscopy (2DES) is a popular technique that can track ultrafast coherent and incoherent processes in real time. Since its development in the late 1990s, 2DES has become a powerful tool for investigating ultrafast dynamics in a range of systems, including nanomaterials and optoelectronic devices. This Primer explains the underlying physical principles of 2DES and how it can be applied to study dynamic photophysical processes. The article discusses how to collect, process and analyse data, with a summary of currently available experimental configurations. Common issues and challenges are considered, focusing on the limitations and reproducibility of the technique, finishing with an exploration of potential future advances and applications.| File | Dimensione | Formato | |
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nosso_2DES_NatRevMethPri_2023.pdf
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Descrizione: This article may be downloaded for personal use only. Any other use requires prior permission of the author and the Springer Nature. This article appeared in Nature Reviews Methods Primers 3, 84 (2023) and may be found at https://doi.org/10.1038/s43586-023-00267-2.
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