: The "on-demand" capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a "smart" material capable of capturing (chemisorption) CO2 from high-purity flue-gas as well as low-concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses.
Graphene Oxide-Arginine Composites: Efficient Dual Function Materials for Integrated CO2 Capture and Conversion
Mantovani, S.;Pintus, A.;Kovtun, A.;Gondolini, A.;Casadio, S.;Sanson, A.;Rancan, M.;Armelao, L.;Melucci, M.;Bandini, M.
2024
Abstract
: The "on-demand" capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a "smart" material capable of capturing (chemisorption) CO2 from high-purity flue-gas as well as low-concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses.| Campo DC | Valore | Lingua |
|---|---|---|
| dc.authority.ancejournal | CHEMSUSCHEM | en |
| dc.authority.orgunit | Istituto di Scienza, Tecnologia e Sostenibilità per lo Sviluppo dei Materiali Ceramici - ISSMC (ex ISTEC) | en |
| dc.authority.orgunit | Istituto per la Sintesi Organica e la Fotoreattivita' - ISOF | en |
| dc.authority.orgunit | Istituto di Chimica della Materia Condensata e di Tecnologie per l'Energia - ICMATE | en |
| dc.authority.people | Mantovani, S. | en |
| dc.authority.people | Pintus, A. | en |
| dc.authority.people | Kovtun, A. | en |
| dc.authority.people | Gondolini, A. | en |
| dc.authority.people | Casadio, S. | en |
| dc.authority.people | Sanson, A. | en |
| dc.authority.people | Marforio, T. D. | en |
| dc.authority.people | Calvaresi, M. | en |
| dc.authority.people | Rancan, M. | en |
| dc.authority.people | Armelao, L. | en |
| dc.authority.people | Bertuzzi, G. | en |
| dc.authority.people | Melucci, M. | en |
| dc.authority.people | Bandini, M. | en |
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| dc.contributor.appartenenza | Istituto di Chimica della Materia Condensata e di Tecnologie per l'Energia - ICMATE | * |
| dc.contributor.appartenenza | Istituto di Scienza, Tecnologia e Sostenibilità per lo Sviluppo dei Materiali Ceramici - ISSMC (ex ISTEC) | * |
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| dc.date.issued | 2024 | - |
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| dc.description.abstract | : The "on-demand" capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a "smart" material capable of capturing (chemisorption) CO2 from high-purity flue-gas as well as low-concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses. | - |
| dc.description.allpeople | Mantovani, S.; Pintus, A.; Kovtun, A.; Gondolini, A.; Casadio, S.; Sanson, A.; Marforio, T. D.; Calvaresi, M.; Rancan, M.; Armelao, L.; Bertuzzi, G.; Melucci, M.; Bandini, M. | - |
| dc.description.allpeopleoriginal | Mantovani, S.; Pintus, A.; Kovtun, A.; Gondolini, A.; Casadio, S.; Sanson, A.; Marforio, T.D.; Calvaresi, M.; Rancan, M.; Armelao, L.; Bertuzzi, G.; Melucci, M.; Bandini, M. | en |
| dc.description.fulltext | restricted | en |
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| dc.identifier.doi | 10.1002/cssc.202301673 | en |
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| dc.subject.keywords | Carbon dioxide | - |
| dc.subject.keywords | Carbon-capture-conversion | - |
| dc.subject.keywords | Computational study | - |
| dc.subject.keywords | Graphene oxide | - |
| dc.subject.keywords | Spectroscopic investigation | - |
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| dc.subject.singlekeyword | Computational study | * |
| dc.subject.singlekeyword | Graphene oxide | * |
| dc.subject.singlekeyword | Spectroscopic investigation | * |
| dc.title | Graphene Oxide-Arginine Composites: Efficient Dual Function Materials for Integrated CO2 Capture and Conversion | en |
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| scopus.description.abstracteng | The “on-demand” capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a “smart” material capable of capturing (chemisorption) CO2 from high-purity flue-gas as well as low-concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses. | * |
| scopus.description.allpeopleoriginal | Mantovani S.; Pintus A.; Kovtun A.; Gondolini A.; Casadio S.; Sanson A.; Marforio T.D.; Calvaresi M.; Rancan M.; Armelao L.; Bertuzzi G.; Melucci M.; Bandini M. | * |
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| scopus.identifier.doi | 10.1002/cssc.202301673 | * |
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| scopus.subject.keywords | Carbon dioxide; Carbon-capture-conversion; Computational study; Graphene oxide; Spectroscopic investigation; | * |
| scopus.title | Graphene Oxide-Arginine Composites: Efficient Dual Function Materials for Integrated CO2 Capture and Conversion | * |
| scopus.titleeng | Graphene Oxide-Arginine Composites: Efficient Dual Function Materials for Integrated CO2 Capture and Conversion | * |
| Appare nelle tipologie: | 01.01 Articolo in rivista | |
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