The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field H applied perpendicularly to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered XY model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength, a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile-to-strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.

Fragile-to-strong glass transition in two-dimensional vortex liquids

Maccari, I.;Benfatto, L.;Castellani, C.;Lorenzana, J.;
2025

Abstract

The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field H applied perpendicularly to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered XY model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength, a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile-to-strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.
2025
Istituto dei Sistemi Complessi - ISC
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Descrizione: Fragile-to-strong glass transition in two-dimensional vortex liquids
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/540463
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