We propose here a new interpretation of recent quasi-elastic neutron scattering (QENS) measurements on water. A line-shape analysis based on a stretched exponential ansatz for the time decay of density fluctuations enabled us to observe an anomalous dependence on the exchanged momentum of relevant relaxation parameters. We discuss this effect and relate it to an a priori uncorrelated anomaly, previously evidenced by diffraction measurements.

On the anomalous behaviour of microscopic diffusion of liquid water

Cunsolo A;Orecchini A;Petrillo C;Sacchetti F
2007

Abstract

We propose here a new interpretation of recent quasi-elastic neutron scattering (QENS) measurements on water. A line-shape analysis based on a stretched exponential ansatz for the time decay of density fluctuations enabled us to observe an anomalous dependence on the exchanged momentum of relevant relaxation parameters. We discuss this effect and relate it to an a priori uncorrelated anomaly, previously evidenced by diffraction measurements.
2007
INFM
X-RAY-SCATTERING
ENHANCED DENSITY-FLUCTUATIONS
ELASTIC NEUTRON-SCATTERING
SUPERCOOLED WATER
RELAXATIONAL DYNAMICS
File in questo prodotto:
Non ci sono file associati a questo prodotto.

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/159749
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus ND
  • ???jsp.display-item.citation.isi??? ND
social impact