We perform extensive MD simulations of two-dimensional systems of hard disks, focusing on the collisional statistical properties. We analyze the distribution functions of velocity, free flight time, and free path length for packing fractions ranging from the fluid to the solid phase. The behaviors of the mean free flight time and path length between subsequent collisions are found to drastically change in the coexistence phase. We show that single-particle dynamical properties behave analogously in collisional and continuous-time representations, exhibiting apparent crossovers between the fluid and the solid phases. We find that, both in collisional and continuous-time representation, the mean-squared displacement, velocity autocorrelation functions, intermediate scattering functions, and self-part of the van Hove function (propagator) closely reproduce the same behavior exhibited by the corresponding quantities in granular media, colloids, and supercooled liquids close to the glass or jamming transition.

Collisional statistics and dynamics of two-dimensional hard-disk systems: From fluid to solid

Alessandro Taloni;
2015

Abstract

We perform extensive MD simulations of two-dimensional systems of hard disks, focusing on the collisional statistical properties. We analyze the distribution functions of velocity, free flight time, and free path length for packing fractions ranging from the fluid to the solid phase. The behaviors of the mean free flight time and path length between subsequent collisions are found to drastically change in the coexistence phase. We show that single-particle dynamical properties behave analogously in collisional and continuous-time representations, exhibiting apparent crossovers between the fluid and the solid phases. We find that, both in collisional and continuous-time representation, the mean-squared displacement, velocity autocorrelation functions, intermediate scattering functions, and self-part of the van Hove function (propagator) closely reproduce the same behavior exhibited by the corresponding quantities in granular media, colloids, and supercooled liquids close to the glass or jamming transition.
2015
Istituto di Chimica della Materia Condensata e di Tecnologie per l'Energia - ICMATE
VELOCITY-AUTOCORRELATION FUNCTION
MODE-COUPLING THEORY
SPATIALLY HETEROGENEOUS DYNAMICS
File in questo prodotto:
File Dimensione Formato  
prod_334461-doc_104187.pdf

solo utenti autorizzati

Descrizione: Collisional statistics and dynamics of two-dimensional hard-disk systems: From fluid to solid
Tipologia: Versione Editoriale (PDF)
Licenza: NON PUBBLICO - Accesso privato/ristretto
Dimensione 3.56 MB
Formato Adobe PDF
3.56 MB Adobe PDF   Visualizza/Apri   Richiedi una copia
1503.08238.pdf

accesso aperto

Descrizione: Collisional statistics and dynamics of two-dimensional hard-disk systems: From fluid to solid
Tipologia: Documento in Pre-print
Licenza: Creative commons
Dimensione 1.71 MB
Formato Adobe PDF
1.71 MB Adobe PDF Visualizza/Apri

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/292534
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 3
  • ???jsp.display-item.citation.isi??? 2
social impact