We study the interplay of electron-electron and electron-phonon interactions in the course of electron-hole bound-state formation for gapped solid-state systems. Adapting the essentially approximation-free diagrammatic Monte Carlo method for the calculation of the optical response, we discuss the absorption of light in correlated electron-phonon systems for the whole interaction and phonon frequency regimes. The spectral function obtained by analytical continuation from the imaginary-time current-current correlation function demonstrates the dressing of excitons by a phonon cloud when the coupling the lattice degrees of freedom becomes increasingly important, where notable differences show up between the adiabatic and antiadiabatic cases.
Optical signatures of exciton polarons from diagrammatic Monte Carlo
De Filippis G;Cataudella V;
2018
Abstract
We study the interplay of electron-electron and electron-phonon interactions in the course of electron-hole bound-state formation for gapped solid-state systems. Adapting the essentially approximation-free diagrammatic Monte Carlo method for the calculation of the optical response, we discuss the absorption of light in correlated electron-phonon systems for the whole interaction and phonon frequency regimes. The spectral function obtained by analytical continuation from the imaginary-time current-current correlation function demonstrates the dressing of excitons by a phonon cloud when the coupling the lattice degrees of freedom becomes increasingly important, where notable differences show up between the adiabatic and antiadiabatic cases.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.