The theoretical understanding of the low-frequency modes in amorphous solids at finite temperature is still incomplete. The study of the relevant modes is obscured by the dressing of interparticle forces by collision-induced momentum transfer that is unavoidable at finite temperatures. Recently, it was proposed that low-frequency modes of vibrations around the thermally averaged configurations deserve special attention. In simple model glasses with bare binary interactions, these included quasilocalized modes whose density of states appears to be universal, depending on the frequencies as D(?)~?4, in agreement with the similar law that is obtained with bare forces at zero temperature. In this paper, we report investigations of a model of silica glass at finite temperature; here the bare forces include binary and ternary interactions. Nevertheless, we can establish the validity of the universal law of the density of quasilocalized modes also in this richer and more realistic model glass.

Universal density of low-frequency states in silica glass at finite temperatures

Zapperi S
2022

Abstract

The theoretical understanding of the low-frequency modes in amorphous solids at finite temperature is still incomplete. The study of the relevant modes is obscured by the dressing of interparticle forces by collision-induced momentum transfer that is unavoidable at finite temperatures. Recently, it was proposed that low-frequency modes of vibrations around the thermally averaged configurations deserve special attention. In simple model glasses with bare binary interactions, these included quasilocalized modes whose density of states appears to be universal, depending on the frequencies as D(?)~?4, in agreement with the similar law that is obtained with bare forces at zero temperature. In this paper, we report investigations of a model of silica glass at finite temperature; here the bare forces include binary and ternary interactions. Nevertheless, we can establish the validity of the universal law of the density of quasilocalized modes also in this richer and more realistic model glass.
2022
Istituto di Chimica della Materia Condensata e di Tecnologie per l'Energia - ICMATE
silica glass
File in questo prodotto:
File Dimensione Formato  
prod_472156-doc_192103.pdf

accesso aperto

Descrizione: Universal density of low-frequency states in silica glass at finite temperatures
Tipologia: Versione Editoriale (PDF)
Dimensione 2.29 MB
Formato Adobe PDF
2.29 MB Adobe PDF Visualizza/Apri

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/445810
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 4
  • ???jsp.display-item.citation.isi??? 4
social impact