Increasing demand for functional materials crucial for advancing new technologies has motivated significant scientific and industrial research efforts. High-entropy materials (HEMs), with tunable properties, are gaining attention for their use in high-frequency transformers, microwave devices, multiferroics, and high-density magnetic memory components. The initial exploration of HEMs started with high-entropy alloys (HASs), such as CrMnFeCoNi, CuCoNiCrAlxFe, and AlCoCrTiZn and paved the way for a multitude of HEM variations, including oxides, oxyfluorides, borides, carbides, nitrides, sulfides, and phosphides. In this study, we fabricated the high-entropy oxide (HEO) compound (Formula presented.) through the solid-state synthesis method. Magnetic measurements at 300 K show ferromagnetic behavior with significant coercivity. At the same time, this novel composition exhibits excellent dielectric properties and shows potential for electronic applications demonstrating that a high-entropy approach can expand the compositional range of rare earth multiferroics and improve the multifunctional properties in multiferroic applications.

Preparation and Characterization of BXFO High-Entropy Oxides

Aziz S.;Monteduro A. G.;Rizzato S.;Leo A.;Maruccio G.
2024

Abstract

Increasing demand for functional materials crucial for advancing new technologies has motivated significant scientific and industrial research efforts. High-entropy materials (HEMs), with tunable properties, are gaining attention for their use in high-frequency transformers, microwave devices, multiferroics, and high-density magnetic memory components. The initial exploration of HEMs started with high-entropy alloys (HASs), such as CrMnFeCoNi, CuCoNiCrAlxFe, and AlCoCrTiZn and paved the way for a multitude of HEM variations, including oxides, oxyfluorides, borides, carbides, nitrides, sulfides, and phosphides. In this study, we fabricated the high-entropy oxide (HEO) compound (Formula presented.) through the solid-state synthesis method. Magnetic measurements at 300 K show ferromagnetic behavior with significant coercivity. At the same time, this novel composition exhibits excellent dielectric properties and shows potential for electronic applications demonstrating that a high-entropy approach can expand the compositional range of rare earth multiferroics and improve the multifunctional properties in multiferroic applications.
2024
Istituto di Nanotecnologia - NANOTEC - Sede Lecce
bismuth ferrite
high-entropy oxides
magnetization
multi-doping
multiferroics
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.14243/537718
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